Quantum-Enhanced Nonlinear Spectroscopy

This thesis focuses on nonlinear spectroscopy from a quantum optics perspective. First, it provides a detailed introduction to nonlinear optical signals; starting from Glauber’s photon counting formalism, it establishes the diagrammatic formulation, which forms the backbone of nonlinear molecular spectroscopy.

 

The main body of the thesis investigates the impact of quantum correlations in entangled...